Thermodynamics Research Center / ThermoML | Journal of Chemical and Engineering Data

Experimental Measurement and Thermodynamic Modeling for the Solubility of Methane in Water and Hexadecane

Campos, C. E. P. S., Penello, J. R., Pessoa, F. L. P., Uller, A. M. C.
J. Chem. Eng. Data 2010, 55, 7, 2576-2580
ABSTRACT
In the petroleum industry, there is direct contact among oil, gases, and water in many steps of petroleum exploitation and refining operations. The main constituent of the natural gas is methane, presenting on its composition 95 % of this substance. To design and optimize these operations a correct characterization of the phase equilibrium is essential, which depends on accurate experimental data and thermodynamic models. So, the main goal of this work was the experimental measurement of methane solubility in water and hexadecane, since this organic compound has properties similar to the average properties of Brazilian heavy oil. The experimental conditions used were a temperature range from (303.2 to 323.2) K and a low pressure range from (60.8 to 638.5) kPa. Moreover, the results were correlated using the best thermodynamic model, the Peng-Robinson equation of state for both phases with original mixing rules, to describe the behavior of the systems, demonstrating satisfactory bubble-point calculation.
Compounds
# Formula Name
1 CH4 methane
2 C16H34 hexadecane
3 H2O water
Datasets
The table above is generated from the ThermoML associated json file (link above). POMD and RXND refer to PureOrMixture and Reaction Datasets. The compound numbers are included in properties, variables, and phases, if specificied; the numbers refer to the table of compounds on the left.
Type Compound-# Property Variable Constraint Phase Method #Points
  • POMD
  • 1
  • 3
  • Mole fraction - 1 ; Liquid
  • Temperature, K; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Gas
  • pressure change or dissolution
  • 18
  • POMD
  • 1
  • 2
  • Mole fraction - 1 ; Liquid
  • Temperature, K; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Gas
  • pressure change or dissolution
  • 18