Thermodynamics Research Center / ThermoML | Journal of Chemical and Engineering Data

Thermophysical Properties of 1-Ethyl-3-methylimidazolium Ethylsulfate and 1-Butyl-3-methylimidazolium Methylsulfate Ionic Liquids

Fernandez, A.[Adela], Torrecilla, J. S.[Jose S.], Rodriquez, F.[Francisco]
J. Chem. Eng. Data 2007, 52, 5, 1979-1983
ABSTRACT
Heat capacity, glass-transition, crystallization, and melting temperatures of 1-ethyl-3-methylimidazolium ethylsulfate ([Emim][EtSO4]) and 1-butyl-3-methylimidazolium methylsulfate ([Bmim][MeSO4]) ionic liquids (ILs) have been determined by differential scanning calorimetry (DSC). Their thermal stabilities have been analyzed by thermogravimetric analysis (TGA). Given the effect of the heating rate over the decomposition temperatures, isothermal TGA experiments are proposed as a more appropriate method to evaluate the thermal stability of the ILs. Inside the working range (-150 deg C to 30 deg C), [Emim][EtSO4] and [Bmim][MeSO4] present a glass-transition temperature of -78.4 deg C and -91.9 deg C, respectively. [Bmim][MeSO4] has a melting temperature of -4.1 deg C. The Cp was determined in a working range (10 deg C to 100 deg C) where its value increases lineally with temperature.
Compounds
# Formula Name
1 C8H16N2O4S 1-ethyl-3-methylimidazolium ethyl sulfate
2 C9H18N2O4S 1-butyl-3-methylimidazolium methyl sulfate
Datasets
The table above is generated from the ThermoML associated json file (link above). POMD and RXND refer to PureOrMixture and Reaction Datasets. The compound numbers are included in properties, variables, and phases, if specificied; the numbers refer to the table of compounds on the left.
Type Compound-# Property Variable Constraint Phase Method #Points
  • POMD
  • 1
  • Triple point temperature, K ; Glass
  • Glass
  • Liquid
  • Air at 1 atmosphere
  • DTA
  • 1
  • POMD
  • 1
  • Molar heat capacity at constant pressure, J/K/mol ; Liquid
  • Temperature, K; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Small sample (50 mg) DSC
  • 10
  • POMD
  • 2
  • Triple point temperature, K ; Glass
  • Glass
  • Liquid
  • Air at 1 atmosphere
  • DTA
  • 1
  • POMD
  • 2
  • Normal melting temperature, K ; Crystal
  • Crystal
  • Liquid
  • Air at 1 atmosphere
  • DTA
  • 1
  • POMD
  • 2
  • Molar heat capacity at constant pressure, J/K/mol ; Liquid
  • Temperature, K; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • SDSC:UFactor:3
  • 10