Thermodynamics Research Center / ThermoML | Journal of Chemical and Engineering Data

Measurement and Modeling of the Solubility of Anthracene and Carbazole in Compressed Isobutane

Martinez, F.[Fabiola], Martin, A.[Alicia], Rincon, J.[Jesusa]
J. Chem. Eng. Data 2012, 57, 11, 2928-2935
ABSTRACT
The solubilities of anthracene and carbazole in liquid and supercritical isobutane have been experimentally determined in a static view cell, at temperatures from (367 to 418 K) and pressures from (3.2 to 8.6) MPa. The solubilities of anthracene varied from (7.3 to 51.8) mg of solute per gram of isobutane, whereas those of carbazole were from (1.4 to 9.9) mg of solute per gram of isobutane within the experimental range studied. These differences in solute solubilities have been explained attending to the higher vapor pressures of anthracene and its smaller dipole moment (and so stronger affinity to isobutane). The experimental solubilities have been compared to those of these solutes in propane and CO2. At similar reduced temperature and pressure conditions, it has been found that solute mole fractions are higher in isobutane than in the other two fluids (3 to 15 times and 160 to 270 times higher than in propane and CO2, respectively). Anthracene and carbazole solubilities in isobutane have been modeled by the Peng Robinson equation of state. Good fit of the experimental results has been obtained (APD values of 6.7 % for anthracene and 9.7 % for carbazole).
Compounds
# Formula Name
1 C4H10 2-methylpropane
2 C14H10 anthracene
3 C12H9N 9H-carbazole
Datasets
The table above is generated from the ThermoML associated json file (link above). POMD and RXND refer to PureOrMixture and Reaction Datasets. The compound numbers are included in properties, variables, and phases, if specificied; the numbers refer to the table of compounds on the left.
Type Compound-# Property Variable Constraint Phase Method #Points
  • POMD
  • 1
  • 2
  • Mole fraction - 2 ; Liquid
  • Temperature, K; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Crystal - 2
  • View cell with pressure adjustment
  • 11
  • POMD
  • 1
  • 3
  • Mole fraction - 3 ; Liquid
  • Temperature, K; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Crystal - 3
  • View cell with pressure adjustment
  • 11