Thermodynamics Research Center / ThermoML | Journal of Chemical and Engineering Data

Experimental Measurement and Modeling of Aniline Hydrochloride Solubility in Water, Methanol, Ethanol, 1- Propanol and Their Mixed Systems

Sun, S.[Shunping], Li, Z.[Zhibao]
J. Chem. Eng. Data 2012, 57, 1, 219-226
ABSTRACT
The solubility of aniline hydrochloride ([HAE]Cl) in different aqueous solutions of methanol, ethanol, 1-propanol and their mixed solvent solutions were determined using dynamic method in the temperature range between 288 K and 328 K. With the purpose of improving AspenPlus s prediction capability, in regard to [HAE]Cl solubilities in the CH3OH C2H5OH C3H7OH H2O system at various temperatures, new interaction energy parameters + - [HAE] -Cl ,CH3OH o + - CH3OH,[HAE] -Cl o , + - [HAE] -Cl ,C2H5OH o + - C2H5OH,[HAE] -Cl o and + - [HAE] -Cl ,C3H7OH o + - C3H7OH,[HAE] -Cl o were obtained via the regression of experimental solubility of [HAE]Cl in binary mixed solvent systems with maximum-likelihood principle. With the electrolyte NRTL (ENRTL) interaction parameters newly obtained, a self-consistent model was established for the calculation of [HAE]Cl solubility in the system of CH3OH C2H5OH C3H7OH H2O as a function of temperature and the composition of solvents. The maximum relative deviation between experimental and predicted solubility data is 2.3% and the average relative deviation is 1.8%.
Compounds
# Formula Name
1 C6H8ClN aniline hydrochloride
2 CH4O methanol
3 C2H6O ethanol
4 C3H8O propan-1-ol
5 H2O water
Datasets
The table above is generated from the ThermoML associated json file (link above). POMD and RXND refer to PureOrMixture and Reaction Datasets. The compound numbers are included in properties, variables, and phases, if specificied; the numbers refer to the table of compounds on the left.
Type Compound-# Property Variable Constraint Phase Method #Points
  • POMD
  • 2
  • 1
  • Mole fraction - 1 ; Liquid
  • Temperature, K; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Crystal - 1
  • Titration method
  • 5
  • POMD
  • 3
  • 1
  • Mole fraction - 1 ; Liquid
  • Temperature, K; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Crystal - 1
  • Titration method
  • 5
  • POMD
  • 4
  • 1
  • Mole fraction - 1 ; Liquid
  • Temperature, K; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Crystal - 1
  • Titration method
  • 5
  • POMD
  • 2
  • 1
  • 5
  • Molality, mol/kg - 1 ; Liquid
  • Temperature, K; Liquid
  • Solvent: Mass fraction - 2; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Crystal - 1
  • Titration
  • 25
  • POMD
  • 3
  • 1
  • 5
  • Molality, mol/kg - 1 ; Liquid
  • Temperature, K; Liquid
  • Solvent: Mass fraction - 3; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Crystal - 1
  • Titration
  • 42
  • POMD
  • 4
  • 1
  • 5
  • Molality, mol/kg - 1 ; Liquid
  • Temperature, K; Liquid
  • Solvent: Mass fraction - 4; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Crystal - 1
  • Titration
  • 30