Thermodynamics Research Center / ThermoML | Journal of Chemical and Engineering Data

Thermochemical Properties of Formamide Revisited: New Experiment and Quantum Mechanical Calculations

Emel'yanenko, V.[Vladimir], Verevkin, S.[Sergey], Varfolomeev, M.[Mikhail]
J. Chem. Eng. Data 2011, 56, 11, 4183-4187
ABSTRACT
Formamide is one of the key compounds in organic chemistry. Surprisingly, the experimental thermochemical data for this compound are scarce. In this work, the standard molar enthalpy of formation in the gaseous state of formamide ?fHmdeg (g, 298.15 K) = (-188.6 +- 0.4) kJ*mol 1 has been derived from enthalpy of formation ?fHmdeg (l, 298.15 K) = (-571.4 +- 0.3) kJ*mol 1 (measured calorimetrically) and the molar enthalpy of vaporization ?1gHm = (62.2 +- 0.3) kJ*mol 1 obtained from the vapor pressure measurements. To verify the experimental data, first-principles calculations have been performed using density functional theory (DFT), MPn, W1U, CBS-n, and Gn methods.
Compounds
# Formula Name
1 CO2 carbon dioxide
2 N2 nitrogen
3 H2O water
4 O2 oxygen
5 CH3NO formamide
Datasets
The table above is generated from the ThermoML associated json file (link above). POMD and RXND refer to PureOrMixture and Reaction Datasets. The compound numbers are included in properties, variables, and phases, if specificied; the numbers refer to the table of compounds on the left.
Type Compound-# Property Variable Constraint Phase Method #Points
  • POMD
  • 5
  • Vapor or sublimation pressure, kPa ; Liquid
  • Temperature, K; Liquid
  • Liquid
  • Gas
  • Transpiration method
  • 17
  • RXND
  • 5
  • 1
  • 2
  • 3
  • 4
  • Specific internal energy of reaction at constant volume, J/g
  • Static bomb calorimetry
  • 1