Thermodynamics Research Center / ThermoML | Journal of Chemical and Engineering Data

Measurement of the Effect of Salt on Vapor-Liquid Equilibria by Using Headspace Gas Chromatography

Takamatsu, H.[Hideaki], Ohe, S.[Shuzo]
J. Chem. Eng. Data 2003, 48, 2, 277-279
ABSTRACT
The effect of salt on vapor-liquid equilibria for ethyl acetate + ethanol + CaCl2 and + LiCl was measured by using headspace gas chromatography (HSGC) at 313.15 K. Applying a HSGC technique to the measurement of VLE has three advantages, namely, a short measurement time, a small sample volume, and minor skills required. As a result, relative volatility was increased with salt concentrations. LiCl showed stronger effect than CaCl2. The observed data were well correlated with a modified solvation model and with an electrolyte NRTL model. The azeptropic points were estimated by the modified solvation model. It was confirmed that the point was observed to shift to the ethyl acetate-rich region in CaCl2 system and that LiCl broke the azeotrope.
Compounds
# Formula Name
1 C4H8O2 ethyl acetate
2 C2H6O ethanol
3 CaCl2 calcium chloride
4 ClLi lithium chloride
Datasets
The table above is generated from the ThermoML associated json file (link above). POMD and RXND refer to PureOrMixture and Reaction Datasets. The compound numbers are included in properties, variables, and phases, if specificied; the numbers refer to the table of compounds on the left.
Type Compound-# Property Variable Constraint Phase Method #Points
  • POMD
  • 2
  • 1
  • Mole fraction - 1 ; Gas
  • Mole fraction - 1; Liquid
  • Temperature, K; Gas
  • Gas
  • Liquid
  • CHROM:UFactor:2
  • 17
  • POMD
  • 2
  • 1
  • 4
  • Mole fraction - 1 ; Gas
  • Mole fraction - 4; Liquid
  • Solvent: Mole fraction - 1; Liquid
  • Temperature, K; Gas
  • Gas
  • Liquid
  • CHROM:UFactor:2
  • 16
  • POMD
  • 2
  • 1
  • 3
  • Mole fraction - 1 ; Gas
  • Mole fraction - 3; Liquid
  • Solvent: Mole fraction - 1; Liquid
  • Temperature, K; Gas
  • Gas
  • Liquid
  • CHROM:UFactor:2
  • 17