Thermodynamics Research Center / ThermoML | Journal of Chemical and Engineering Data

Thermodynamic Properties of Octamethylcyclotetrasiloxane

Thol, M.[Monika], Rutkai, G.[Gabor], Koster, A.[Andreas], Dubberke, F. H.[Frithjof H.], Windmann, T.[Thorsten], Span, R.[Roland], Vrabec, J.[Jadran]
J. Chem. Eng. Data 2016, 61, 7, 2580-2595
ABSTRACT
An equation of state for octamethylcyclotetrasiloxane is presented. The available experimental data from the literature are supplemented by new measurements on the speed of sound. Furthermore, a new force field is proposed, allowing the generation of a comprehensive thermodynamic data set by means of molecular simulation. Both the experimental and molecular simulation data are applied to develop a fundamental equation of state in terms of the Helmholtz energy. On the basis of the experimental data, the equation of state is valid from the triple-point temperature to T = 590 K for pressures up to p = 180 MPa and can be used to calculate any thermodynamic equilibrium state property. Its accuracy is assessed by a comprehensive analysis of the underlying experimental data. Finally, the range of validity was extended to Tmax = 1200 K and pmax = 520 MPa by means of molecular simulation data.
Compounds
# Formula Name
1 C8H24O4Si4 octamethylcyclotetrasiloxane
Datasets
The table above is generated from the ThermoML associated json file (link above). POMD and RXND refer to PureOrMixture and Reaction Datasets. The compound numbers are included in properties, variables, and phases, if specificied; the numbers refer to the table of compounds on the left.
Type Compound-# Property Variable Constraint Phase Method #Points
  • POMD
  • 1
  • Speed of sound, m/s ; Liquid
  • Temperature, K; Liquid
  • Pressure, kPa; Liquid
  • Frequency, MHz; Liquid
  • Liquid
  • Pulse-echo method
  • 54