Thermodynamics Research Center / ThermoML | Journal of Chemical and Engineering Data

Solubility of Carbon Dioxide in LiF Li2CO3 Molten Salt System

Shi, Z.[Zhongning], Deng, W.[Wentao], Song, X.[Xiaowen], Hu, X.[Xianwei], Gao, B.[Bingliang], Wang, Z.[Zhaowen]
J. Chem. Eng. Data 2016, 61, 9, 3020-3026
ABSTRACT
The solubility of carbon dioxide in a LiF Li2CO3 molten salt system was determined using a pressure differential method. With increasing holding temperature, the solubility of CO2 in LiF Li2CO3 melts decreases rapidly. The influence of the alkali metal fluoride of XF(X = K, Na) content from 5% to 25% on the CO2 solubility was considered. The CO2 solubility in LiF Li2CO3 XF melts decreased with increasing temperature and concentration of XF. The calculated thermodynamic data for CO2 dissolved in these melts revealed that the reaction between CO2 and a carbonate ion was exothermic. At 630 deg C, KF decreased the CO2 solubility more effectively than NaF. When the mole fraction of LiF was 50% in LiF Li2CO3, the CO2 solubility reached a maximum of 6.8 * 10 4 (molCO2/molmelt) at 640 deg C.
Compounds
# Formula Name
1 FLi lithium fluoride
2 CLi2O3 lithium carbonate
3 CO2 carbon dioxide
Datasets
The table above is generated from the ThermoML associated json file (link above). POMD and RXND refer to PureOrMixture and Reaction Datasets. The compound numbers are included in properties, variables, and phases, if specificied; the numbers refer to the table of compounds on the left.
Type Compound-# Property Variable Constraint Phase Method #Points
  • POMD
  • 2
  • Vapor or sublimation pressure, kPa ; Crystal
  • Temperature, K; Crystal
  • Crystal
  • Gas
  • Closed cell (Static) method
  • 1
  • POMD
  • 3
  • 2
  • 1
  • Amount ratio of solute to solvent - 3 ; Liquid
  • Solvent: Mole fraction - 1; Liquid
  • Temperature, K; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Gas
  • phase equilibration
  • 15