Thermodynamics Research Center / ThermoML | Journal of Chemical Thermodynamics

Liquid-liquid equilibrium of alcohol-ester systems with deep eutectic solvent on the base of choline chloride

Samarov, Artemiy, Shner, Natalia, Mozheeva, Ekaterina, Toikka, Alexander
J. Chem. Thermodyn. 2019, 131, 369-374
ABSTRACT
The liquid-liquid equilibrium (LLE) for the mixtures of ethanol - ethyl propionate, n-propanol - n-propyl propionate and n-butanol - n-butyl propionate with deep eutectic solvents (DES) was studied. DES was used on the basis of choline chloride with malonic acid in a mole ratioof 1:1. The studies were carried out at two temperatures, 293.15 K and 313.15 K and atmospheric pressure. The compositions of the coexisting organic and DES phases were determined. On the basis of experimental data, alcohol distribution coefficient and selectivity were calculated and analysed. The effect of the temperature and length of the alcohol alkyl chain on the alcohol distribution coefficient and selectivity were established. Using the non-random two liquids model (NRTL), a thermodynamic simulation of obtained experimental data on the liquid-liquid phase equilibrium was carried out.
Compounds
# Formula Name
1 C5H10O2 ethyl propanoate
2 C6H12O2 propyl propanoate
3 C3H4O4 propanedioic acid
4 C5H14ClNO choline chloride
Datasets
The table above is generated from the ThermoML associated json file (link above). POMD and RXND refer to PureOrMixture and Reaction Datasets. The compound numbers are included in properties, variables, and phases, if specificied; the numbers refer to the table of compounds on the left.
Type Compound-# Property Variable Constraint Phase Method #Points
  • POMD
  • 1
  • 3
  • 4
  • Mass fraction - 1 ; Liquid mixture 1
  • Temperature, K; Liquid mixture 1
  • Pressure, kPa; Liquid mixture 1
  • Solvent: Mole fraction - 3; Liquid mixture 1
  • Liquid mixture 1
  • Liquid mixture 2
  • Chromatography
  • 2
  • POMD
  • 2
  • 3
  • 4
  • Mass fraction - 2 ; Liquid mixture 1
  • Temperature, K; Liquid mixture 1
  • Pressure, kPa; Liquid mixture 1
  • Solvent: Mole fraction - 3; Liquid mixture 1
  • Liquid mixture 1
  • Liquid mixture 2
  • Chromatography
  • 2