Thermodynamics Research Center / ThermoML | Journal of Chemical Thermodynamics

Standard volumetric properties of a chiral pharmaceutical Albicar in water H/D isotopologues in the temperature range from (278.15 to 318.15) K and at ambient pressure

Ivanov, E. V.[Evgeniy V.], Lebedeva, E. Y.[Elena Yu.], Kravchenko, A. N.[Angelina N.]
J. Chem. Thermodyn. 2017, 115, 148-155
ABSTRACT
Densities of solutions of the chiral (in the racemic form) trans-dimethyldiethylglycoluril (1,4-diethyl-3,6- dimethyltetrahydroimidazo[4,5-d]imidazole-2,5(1H,3H)-dione), being a promising tranquilizer Albicar, in ordinary (H2O) and heavy (D2O) water were measured using the Anton Paar DMA 5000 M highprecision vibrating tube densimeter. All experiments were performed within the temperature range between 278.15 K and 318.15 K (with a step of 10 K) at the pressure to be ca. 99.6 kPa. The solution aquamolality was ranged from ca. 0.02 to ca. 0.2 mol (55.51 mol of solvent) 1 for each of H/D isotopically distinguishable systems compared. The standard (partial at infinite dilution) molar volumes as well as expansibilities of the solute were derived from the solution density data. The behavior of solvent isotope effects (IEs) on the considered quantities were described taking account of structure- and interactionrelated features of H2O and D2O media. It was confirmed that the Albicar hydration is enhanced overall in the D2O medium. The volumetric characteristics for the heterocyclic solute being studied were discussed in comparison with those for Mebicar (1,3,4,6-tetramethyl-derivative) and Bicaret (1,3,4,6-tetrae thyl-derivative), using the previous our results.
Compounds
# Formula Name
1 C10H18N4O2 rac-(3aS,6aS)-1,4-diethyl-3,6-dimethyltetrahydroimidazo[4,5-d]imidazole-2,5(1H,3H)-dione
2 D2O water-d2
3 H2O water
Datasets
The table above is generated from the ThermoML associated json file (link above). POMD and RXND refer to PureOrMixture and Reaction Datasets. The compound numbers are included in properties, variables, and phases, if specificied; the numbers refer to the table of compounds on the left.
Type Compound-# Property Variable Constraint Phase Method #Points
  • POMD
  • 2
  • Mass density, kg/m3 ; Liquid
  • Temperature, K; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Vibrating tube method
  • 5
  • POMD
  • 3
  • Mass density, kg/m3 ; Liquid
  • Temperature, K; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Vibrating tube method
  • 5
  • POMD
  • 3
  • 1
  • Mass density, kg/m3 ; Liquid
  • Temperature, K; Liquid
  • Molality, mol/kg - 1; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Vibrating tube method
  • 50
  • POMD
  • 2
  • 1
  • Mass density, kg/m3 ; Liquid
  • Temperature, K; Liquid
  • Molality, mol/kg - 1; Liquid
  • Pressure, kPa; Liquid
  • Liquid
  • Vibrating tube method
  • 50