Thermodynamics Research Center / ThermoML | Journal of Chemical Thermodynamics

Phase behaviour of pseudo-binary systems of pressurized ((propane + L,L-lactide)) at different ethanol to L,L-lactide mole ratios

Bender, J. P.[Joao P.], Tres, M. V.[Marcus V.], Corazza, M. L.[Marcos L.], Ferreira, S. R. S.[Sandra R. S.], Oliveira, J. V.
J. Chem. Thermodyn. 2014, 78, 120-127
ABSTRACT
This work reports phase equilibrium data of pressurized (propane + L,L-lactide) system at different ethanol to monomer mole ratios (9:1; 7:1; 5:1). Phase equilibrium experiments were accomplished in a high-pressure variable-volume view cell employing the static synthetic method. (Vapour + liquid) equilibrium data for the pseudo-binary systems were determined within the temperature range from (323 to 353) K and pressures up to 3.3 MPa. For the systems investigated, (vapour + liquid) equilibrium (VLE) was visually recorded. It was observed that an increase in temperature or in propane concentration led to a pronounced rise in pressure transition values. On the other hand, an increase in the ethanol to L,L-lactide mole ratio led to a reduction in pressure transitions, whereas a reduction in ethanol concentration complicates the achievement of one-phase homogeneous system. Thus, rapid complete miscibility of the system can be controlled by the amount of ethanol added as a co-solvent. The experimental results were modelled using the Peng Robinson (PR) equation of state with the Wong Sandler (PR WS) mixing rule, providing a good representation of the experimental phase transition points.
Compounds
# Formula Name
1 C6H8O4 (3S,6S)-3,6-dimethyl-1,4-dioxane-2,5-dione
2 C3H8 propane
3 C2H6O ethanol
Datasets
The table above is generated from the ThermoML associated json file (link above). POMD and RXND refer to PureOrMixture and Reaction Datasets. The compound numbers are included in properties, variables, and phases, if specificied; the numbers refer to the table of compounds on the left.
Type Compound-# Property Variable Constraint Phase Method #Points
  • POMD
  • 3
  • 2
  • 1
  • Vapor or sublimation pressure, kPa ; Liquid
  • Temperature, K; Liquid
  • Solvent: Mole fraction - 3; Liquid
  • Mole fraction - 2; Liquid
  • Liquid
  • Gas
  • Variable-volume view cell
  • 97