Thermodynamics Research Center / ThermoML | Journal of Chemical Thermodynamics

Energetics of 1-(aminophenyl)pyrroles: A joint calorimetric and computational study

Santos, A. F. L. O. M.[Ana Filipa L.O.M.], da Silva, M. A. V. R.[Manuel A. V. Ribeiro]
J. Chem. Thermodyn. 2011, 43, 10, 1480-1487
ABSTRACT
Static bomb calorimetry and the Knudsen effusion mass-loss technique were used to derive, respectively, the standard (p = 0.1 MPa) molar enthalpy of formation, in the crystalline phase and the standard molar enthalpy of sublimation, at T = 298.15 K of 1-(2-aminophenyl)pyrrole. These experiments allowed the determination of its standard (p = 0.1 MPa) molar enthalpy of formation, in the gaseous phase, at T = 298.15 K, as (224.1 +- 2.4) kJ mol-1. The gas-phase enthalpy of formation of 1-(2-aminophenyl)pyrrole was also estimated by G3(MP2)// B3LYP calculations, which were further extended to the (aminophenyl)pyrroles that were not studied experimentally. Experimental and theoretical results are in very good agreement.
Compounds
# Formula Name
1 H2 hydrogen
2 N2 nitrogen
3 C graphite
4 CO2 carbon dioxide
5 H2O water
6 O2 oxygen
7 C10H10N2 1-(2-aminophenyl)pyrrole
Datasets
The table above is generated from the ThermoML associated json file (link above). POMD and RXND refer to PureOrMixture and Reaction Datasets. The compound numbers are included in properties, variables, and phases, if specificied; the numbers refer to the table of compounds on the left.
Type Compound-# Property Variable Constraint Phase Method #Points
  • POMD
  • 7
  • Molar enthalpy of vaporization or sublimation, kJ/mol ; Crystal
  • Temperature, K; Crystal
  • Crystal
  • Gas
  • Second Law analysis of vapor pressure data
  • 1
  • POMD
  • 7
  • Vapor or sublimation pressure, kPa ; Crystal
  • Temperature, K; Crystal
  • Crystal
  • Gas
  • Calculated from knudsen effusion weight loss
  • 36
  • RXND
  • 7
  • 1
  • 2
  • 3
  • Molar enthalpy of reaction, kJ/mol
  • Static bomb calorimetry
  • 1
  • RXND
  • 7
  • 4
  • 2
  • 5
  • 6
  • Specific internal energy of reaction at constant volume, J/g
  • Static bomb calorimetry
  • 1