Thermodynamics Research Center / ThermoML | International Journal of Thermophysics

The Phase Transition in a Hybrid Layered Perovskite: [NH3-(CH2)10NH3]ZnCl4 of 1,10-Diaminodecane

Kaiba, A.
Int. J. Thermophys. 2019, 40, 8, 73
ABSTRACT
We investigated the synthesis and structural phase transition of a zero-dimensional organic inorganic hybrid family (NH3C10H20NH3) ZnCl4 by systematic characterizations. This composite revealed a reversible first-order isostructural phase transition from space group P-1 (Phase II) to space group P-1 (Phase I) at round T 358 K. The phase transition can be ascribed to the order disorder transition of the 1,10-Diaminodecane cations. It is known that the interesting electronic and optical properties in this family are dominated by the inorganic parts. The phase transition observed in this work arises from the organic parts. One of the main objectives is to forge a relationship between structural and thermal properties. Thus, adapting the organic fragments can lead to new multifunctional materials. A more in-depth analysis of the structural properties demonstrates the role played by the organic parts in the phase transition shown by the titled compound.
Compounds
# Formula Name
1 C10H26Cl4N2Zn decane-1,10-diaminium tetrachlorozincate(II)
Datasets
The table above is generated from the ThermoML associated json file (link above). POMD and RXND refer to PureOrMixture and Reaction Datasets. The compound numbers are included in properties, variables, and phases, if specificied; the numbers refer to the table of compounds on the left.
Type Compound-# Property Variable Constraint Phase Method #Points
  • POMD
  • 1
  • Triple point temperature, K ; Crystal 2
  • Crystal 2
  • Crystal 1
  • Air at 1 atmosphere
  • X-ray diffraction
  • 1
  • POMD
  • 1
  • Mass density, kg/m3 ; Crystal 2
  • Temperature, K; Crystal 2
  • Pressure, kPa; Crystal 2
  • Crystal 2
  • X-ray diffraction
  • 2