2
0
2009
muh
mut
0
journal
Original
Muhammad, A.[Ayyaz]
Mutalib, M. I. A.[Mohamed I. Abdul]
Murugesan, T.[Thanabalan]
Shafeeq, A.[Amir]
J. Chem. Eng. Data
2009
2020-09-29
Thermophysical Properties of Aqueous Piperazine and Aqueous (N-Methyldiethanolamine + Piperazine) Solutions at Temperatures (298.15 to 338.15) K
In the present work, thermophysical properties such as density (F), dynamic viscosity (c), refractive index (nD), and surface tension (o) of aqueous piperazine (PZ) solutions with mass fractions (100w ) 1.74, 5.16, 10.35) have been measured from temperatures (298.15 to 338.15) K. All of these properties have also been measured for the aqueous blends of N-methyldiethanolamine (MDEA) and piperazine (PZ) with mass fractions {100(w1/w2) ) 32.28/1.74, 32.28/5.16, 32.28/10.35, 48.80/1.74, 48.80/5.16, 48.80/10.35)} for the entire temperature range. The limit of PZ solubility in water was measured by the addition of a known quantity of anhydrous PZ (solid crystals) in 20 mL of distilled water at temperatures (278 to 343) K with a regular interval of 5 K. The experimental values of the studied physical properties have been compared with the literature and also correlated as a function of temperature. The coefficients of thermal expansion (Rp) values have been calculated from their experimental density data using an empirical correlation. A thermogravimetric analyzer (TGA) has been used to explore the thermal stability of the studied solvent systems at a heating rate of 10 deg C* min-1.
10.1021/je9000069
8
54
2317-2321
1
InChI=1S/C5H13NO2/c1-6(2-4-7)3-5-8/h7-8H,2-5H2,1H3
CRVGTESFCCXCTH-UHFFFAOYSA-N
N-methyldiethanolamine
2,2'-(methylazanediyl)bis(ethan-1-ol)
2,2'-methyliminodiethanol
MDEA
methyldiethanolamine
C5H13NO2
1
Commercial source
1
99.5
3
Gas chromatography
2
None used
2
InChI=1S/C4H10N2/c1-2-6-4-3-5-1/h5-6H,1-4H2
GLUUGHFHXGJENI-UHFFFAOYSA-N
piperazine
diethylenediamine
hexahydro-1,4-diazine
hexahydropyrazine
C4H10N2
1
Commercial source
1
99.9
3
Gas chromatography
2
None used
3
InChI=1S/H2O/h1H2
XLYOFNOQVPJJNP-UHFFFAOYSA-N
water
H2O
1
Commercial source
1
99.9
3
Estimated by the compiler
1
2
1
3
1
Principal objective of the work
VVD
TRC
5/29/2014
1
Mole fraction
Titration method
2
Liquid
Direct value, X
1
Data file compiler
Propagation of evaluated standard uncertainties
95
Liquid
Crystal
2
1
Pressure, kPa
Liquid
101
3
1
Temperature, K
Liquid
1
318
3
1
0.124
3
1
0.001
1
323
3
1
0.127
3
1
0.001
1
328
3
1
0.13
3
1
0.001
1
333
3
1
0.132
3
1
0.001
1
338
3
1
0.134
3
1
0.001
1
343
3
1
0.136
3
1
0.001
1
313
3
1
0.121
3
1
0.001
2
2
1
3
1
Principal objective of the work
VVD
TRC
5/29/2014
1
Mole fraction
Titration method
2
Liquid
Direct value, X
1
Data file compiler
Propagation of evaluated standard uncertainties
95
Liquid
Crystal of intercomponent compound 1
1
Pressure, kPa
Liquid
101
3
1
Temperature, K
Liquid
1
278
3
1
0.015
2
1
0.001
1
283
3
1
0.022
2
1
0.001
1
288
3
1
0.025
2
1
0.001
1
293
3
1
0.03
2
1
0.001
1
298
3
1
0.034
2
1
0.001
3
2
1
3
1
Principal objective of the work
JAB
TRC
8/19/2009
1
Surface tension liquid-gas, N/m
Ring tensiometer
Liquid
Direct value, X
1
Data file compiler
Propagation of evaluated standard uncertainties
95
Liquid
Air at 1 atmosphere
1
Temperature, K
Liquid
2
Mass fraction
2
Liquid
1
303.1
4
2
0.0174
3
1
0.07148
4
1
0.00091
1
303.1
4
2
0.0516
3
1
0.07024
4
1
0.0009
1
303.1
4
2
0.1035
4
1
0.0691
4
1
0.00088
1
313.2
4
2
0.0174
3
1
0.06934
4
1
0.00088
1
313.2
4
2
0.0516
3
1
0.06851
4
1
0.00087
1
313.2
4
2
0.1035
4
1
0.06792
4
1
0.00087
1
318.2
4
2
0.0174
3
1
0.06876
4
1
0.00088
1
318.2
4
2
0.0516
3
1
0.06735
4
1
0.00086
1
318.2
4
2
0.1035
4
1
0.06675
4
1
0.00086
1
323.1
4
2
0.0174
3
1
0.06784
4
1
0.00087
1
323.1
4
2
0.0516
3
1
0.0667
4
1
0.00085
1
323.1
4
2
0.1035
4
1
0.06537
4
1
0.00084
1
333.3
4
2
0.0174
3
1
0.06621
4
1
0.00085
1
333.3
4
2
0.0516
3
1
0.06526
4
1
0.00084
1
333.3
4
2
0.1035
4
1
0.06414
4
1
0.00082
4
2
1
3
1
Principal objective of the work
JAB
TRC
8/19/2009
1
Viscosity, Pa*s
CAPTUB:UFactor:8
Liquid
Direct value, X
1
Data file compiler
Propagation of evaluated standard uncertainties
95
Liquid
1
Pressure, kPa
Liquid
101
3
1
Temperature, K
Liquid
2
Mass fraction
2
Liquid
1
303.15
5
2
0.0174
3
1
0.00086
2
1
4e-05
1
303.15
5
2
0.0516
3
1
0.00097
2
1
5e-05
1
303.15
5
2
0.1035
4
1
0.00128
3
1
6e-05
1
313.15
5
2
0.0174
3
1
0.00069
2
1
4e-05
1
313.15
5
2
0.0516
3
1
0.00076
2
1
4e-05
1
313.15
5
2
0.1035
4
1
0.00102
3
1
5e-05
1
318.15
5
2
0.0174
3
1
0.00061
2
1
3e-05
1
318.15
5
2
0.0516
3
1
0.00069
2
1
4e-05
1
318.15
5
2
0.1035
4
1
0.00092
2
1
5e-05
1
323.15
5
2
0.0174
3
1
0.00057
2
1
3e-05
1
323.15
5
2
0.0516
3
1
0.00062
2
1
3e-05
1
323.15
5
2
0.1035
4
1
0.00081
2
1
4e-05
1
333.15
5
2
0.0174
3
1
0.00047
2
1
3e-05
1
333.15
5
2
0.0516
3
1
0.00051
2
1
3e-05
1
333.15
5
2
0.1035
4
1
0.00059
2
1
3e-05
5
2
1
3
1
Principal objective of the work
JAB
TRC
8/19/2009
1
Refractive index (Na D-line)
ABBE:UFactor:4
Liquid
Direct value, X
1
Data file compiler
Propagation of evaluated standard uncertainties
95
Liquid
1
Pressure, kPa
Liquid
101
3
1
Temperature, K
Liquid
2
Mass fraction
2
Liquid
1
303.15
5
2
0.0174
3
1
1.33449
6
1
0.00124
1
303.15
5
2
0.0516
3
1
1.34019
6
1
0.00124
1
303.15
5
2
0.1035
4
1
1.34847
6
1
0.00124
1
313.15
5
2
0.0174
3
1
1.33366
6
1
0.00124
1
313.15
5
2
0.0516
3
1
1.33914
6
1
0.00124
1
313.15
5
2
0.1035
4
1
1.34797
6
1
0.00124
1
318.15
5
2
0.0174
3
1
1.33324
6
1
0.00124
1
318.15
5
2
0.0516
3
1
1.33831
6
1
0.00124
1
318.15
5
2
0.1035
4
1
1.34752
6
1
0.00124
1
323.15
5
2
0.0174
3
1
1.33287
6
1
0.00124
1
323.15
5
2
0.0516
3
1
1.33793
6
1
0.00124
1
323.15
5
2
0.1035
4
1
1.34699
6
1
0.00124
1
333.15
5
2
0.0174
3
1
1.33241
6
1
0.00124
1
333.15
5
2
0.0516
3
1
1.33638
6
1
0.00124
1
333.15
5
2
0.1035
4
1
1.34632
6
1
0.00124
6
2
1
3
1
Principal objective of the work
JAB
TRC
8/19/2009
1
Mass density, kg/m3
VIBTUB:UFactor:16
Liquid
Direct value, X
1
Data file compiler
Propagation of evaluated standard uncertainties
95
Liquid
1
Pressure, kPa
Liquid
101
3
1
Temperature, K
Liquid
2
Mass fraction
2
Liquid
1
298.15
5
2
0.0174
3
1
998.287
6
1
0.508
1
298.15
5
2
0.0516
3
1
999.36
6
1
0.502
1
298.15
5
2
0.1035
4
1
1001.285
7
1
0.506
1
303.15
5
2
0.0174
3
1
996.868
6
1
0.517
1
303.15
5
2
0.0516
3
1
997.913
6
1
0.511
1
303.15
5
2
0.1035
4
1
999.758
6
1
0.499
1
308.15
5
2
0.0174
3
1
995.233
6
1
0.528
1
308.15
5
2
0.0516
3
1
996.252
6
1
0.521
1
308.15
5
2
0.1035
4
1
998.022
6
1
0.51
1
313.15
5
2
0.0174
3
1
993.399
6
1
0.539
1
313.15
5
2
0.0516
3
1
994.396
6
1
0.533
1
313.15
5
2
0.1035
4
1
996.095
6
1
0.522
1
318.15
5
2
0.0174
3
1
991.382
6
1
0.552
1
318.15
5
2
0.0516
3
1
992.359
6
1
0.546
1
318.15
5
2
0.1035
4
1
993.991
6
1
0.535
1
323.15
5
2
0.0174
3
1
989.188
6
1
0.566
1
323.15
5
2
0.0516
3
1
990.147
6
1
0.56
1
323.15
5
2
0.1035
4
1
991.722
6
1
0.55
1
328.15
5
2
0.0174
3
1
986.804
6
1
0.581
1
328.15
5
2
0.0516
3
1
987.769
6
1
0.575
1
328.15
5
2
0.1035
4
1
989.288
6
1
0.565
1
333.15
5
2
0.0174
3
1
984.32
6
1
0.596
1
333.15
5
2
0.0516
3
1
985.241
6
1
0.591
1
333.15
5
2
0.1035
4
1
986.131
6
1
0.585
1
338.15
5
2
0.0174
3
1
981.667
6
1
0.613
1
338.15
5
2
0.0516
3
1
982.506
6
1
0.608
1
338.15
5
2
0.1035
4
1
983.952
6
1
0.599
7
1
1
2
1
3
1
Principal objective of the work
JAB
TRC
8/19/2009
1
Surface tension liquid-gas, N/m
Ring tensiometer
Liquid
Direct value, X
1
Data file compiler
Propagation of evaluated standard uncertainties
95
Liquid
Air at 1 atmosphere
1
Temperature, K
Liquid
2
Mass fraction
1
Liquid
3
Mass fraction
2
Liquid
1
303.1
4
2
0.3228
4
3
0.0174
3
1
0.06032
4
1
0.00078
1
303.1
4
2
0.3228
4
3
0.0516
3
1
0.0597
4
1
0.00077
1
303.1
4
2
0.3228
4
3
0.1035
4
1
0.05886
4
1
0.00076
1
303.1
4
2
0.488
4
3
0.0174
3
1
0.05752
4
1
0.00075
1
303.1
4
2
0.488
4
3
0.0516
3
1
0.05672
4
1
0.00074
1
303.1
4
2
0.488
4
3
0.1035
4
1
0.05623
4
1
0.00074
1
313.2
4
2
0.3228
4
3
0.0174
3
1
0.05886
4
1
0.00076
1
313.2
4
2
0.3228
4
3
0.0516
3
1
0.05832
4
1
0.00076
1
313.2
4
2
0.3228
4
3
0.1035
4
1
0.0579
4
1
0.00075
1
313.2
4
2
0.488
4
3
0.0174
3
1
0.05613
4
1
0.00073
1
313.2
4
2
0.488
4
3
0.0516
3
1
0.0555
4
1
0.00073
1
313.2
4
2
0.488
4
3
0.1035
4
1
0.05522
4
1
0.00072
1
318.2
4
2
0.3228
4
3
0.0174
3
1
0.05814
4
1
0.00076
1
318.2
4
2
0.3228
4
3
0.0516
3
1
0.0576
4
1
0.00075
1
318.2
4
2
0.3228
4
3
0.1035
4
1
0.05681
4
1
0.00074
1
318.2
4
2
0.488
4
3
0.0174
3
1
0.05536
4
1
0.00073
1
318.2
4
2
0.488
4
3
0.0516
3
1
0.05482
4
1
0.00072
1
318.2
4
2
0.488
4
3
0.1035
4
1
0.05438
4
1
0.00071
1
323.1
4
2
0.3228
4
3
0.0174
3
1
0.05763
4
1
0.00075
1
323.1
4
2
0.3228
4
3
0.0516
3
1
0.05706
4
1
0.00074
1
323.1
4
2
0.3228
4
3
0.1035
4
1
0.05623
4
1
0.00073
1
323.1
4
2
0.488
4
3
0.0174
3
1
0.05462
4
1
0.00072
1
323.1
4
2
0.488
4
3
0.0516
3
1
0.05414
4
1
0.00071
1
323.1
4
2
0.488
4
3
0.1035
4
1
0.05367
4
1
0.00071
1
333.3
4
2
0.3228
4
3
0.0174
3
1
0.05644
4
1
0.00074
1
333.3
4
2
0.3228
4
3
0.0516
3
1
0.05585
4
1
0.00073
1
333.3
4
2
0.3228
4
3
0.1035
4
1
0.05532
4
1
0.00072
1
333.3
4
2
0.488
4
3
0.0174
3
1
0.05372
4
1
0.00071
1
333.3
4
2
0.488
4
3
0.0516
3
1
0.05305
4
1
0.0007
1
333.3
4
2
0.488
4
3
0.1035
4
1
0.05249
4
1
0.00069
8
1
1
2
1
3
1
Principal objective of the work
JAB
TRC
8/19/2009
1
Viscosity, Pa*s
CAPTUB:UFactor:8
Liquid
Direct value, X
1
Data file compiler
Propagation of evaluated standard uncertainties
95
Liquid
1
Pressure, kPa
Liquid
101
3
1
Temperature, K
Liquid
2
Mass fraction
1
Liquid
3
Mass fraction
2
Liquid
1
303.15
5
2
0.3228
4
3
0.0174
3
1
0.00362
3
1
0.00016
1
303.15
5
2
0.3228
4
3
0.0516
3
1
0.00411
3
1
0.00018
1
303.15
5
2
0.3228
4
3
0.1035
4
1
0.00562
3
1
0.00024
1
303.15
5
2
0.488
4
3
0.0174
3
1
0.00693
3
1
0.00028
1
303.15
5
2
0.488
4
3
0.0516
3
1
0.00863
3
1
0.00033
1
303.15
5
2
0.488
4
3
0.1035
4
1
0.01174
4
1
0.00043
1
313.15
5
2
0.3228
4
3
0.0174
3
1
0.00248
3
1
0.00011
1
313.15
5
2
0.3228
4
3
0.0516
3
1
0.00297
3
1
0.00013
1
313.15
5
2
0.3228
4
3
0.1035
4
1
0.00404
3
1
0.00018
1
313.15
5
2
0.488
4
3
0.0174
3
1
0.00502
3
1
0.00022
1
313.15
5
2
0.488
4
3
0.0516
3
1
0.00623
3
1
0.00026
1
313.15
5
2
0.488
4
3
0.1035
4
1
0.00841
3
1
0.00032
1
318.15
5
2
0.3228
4
3
0.0174
3
1
0.0022
2
1
0.0001
1
318.15
5
2
0.3228
4
3
0.0516
3
1
0.00267
3
1
0.00012
1
318.15
5
2
0.3228
4
3
0.1035
4
1
0.00357
3
1
0.00016
1
318.15
5
2
0.488
4
3
0.0174
3
1
0.00438
3
1
0.00019
1
318.15
5
2
0.488
4
3
0.0516
3
1
0.00555
3
1
0.00023
1
318.15
5
2
0.488
4
3
0.1035
4
1
0.0074
2
1
0.0003
1
323.15
5
2
0.3228
4
3
0.0174
3
1
0.00196
3
1
9e-05
1
323.15
5
2
0.3228
4
3
0.0516
3
1
0.00238
3
1
0.00011
1
323.15
5
2
0.3228
4
3
0.1035
4
1
0.00294
3
1
0.00013
1
323.15
5
2
0.488
4
3
0.0174
3
1
0.00362
3
1
0.00016
1
323.15
5
2
0.488
4
3
0.0516
3
1
0.00456
3
1
0.0002
1
323.15
5
2
0.488
4
3
0.1035
4
1
0.00628
3
1
0.00026
1
333.15
5
2
0.3228
4
3
0.0174
3
1
0.00132
3
1
6e-05
1
333.15
5
2
0.3228
4
3
0.0516
3
1
0.00172
3
1
8e-05
1
333.15
5
2
0.3228
4
3
0.1035
4
1
0.00221
3
1
0.0001
1
333.15
5
2
0.488
4
3
0.0174
3
1
0.00273
3
1
0.00012
1
333.15
5
2
0.488
4
3
0.0516
3
1
0.00342
3
1
0.00015
1
333.15
5
2
0.488
4
3
0.1035
4
1
0.00462
3
1
0.0002
9
1
1
2
1
3
1
Principal objective of the work
JAB
TRC
8/19/2009
1
Refractive index (Na D-line)
ABBE:UFactor:4
Liquid
Direct value, X
1
Data file compiler
Propagation of evaluated standard uncertainties
95
Liquid
1
Pressure, kPa
Liquid
101
3
1
Temperature, K
Liquid
2
Mass fraction
1
Liquid
3
Mass fraction
2
Liquid
1
303.15
5
2
0.3228
4
3
0.0174
3
1
1.36487
6
1
0.00124
1
303.15
5
2
0.3228
4
3
0.0516
3
1
1.37197
6
1
0.00124
1
303.15
5
2
0.3228
4
3
0.1035
4
1
1.37818
6
1
0.00124
1
303.15
5
2
0.488
4
3
0.0174
3
1
1.37118
6
1
0.00124
1
303.15
5
2
0.488
4
3
0.0516
3
1
1.37752
6
1
0.00124
1
303.15
5
2
0.488
4
3
0.1035
4
1
1.38286
6
1
0.00124
1
313.15
5
2
0.3228
4
3
0.0174
3
1
1.35989
6
1
0.00124
1
313.15
5
2
0.3228
4
3
0.0516
3
1
1.36458
6
1
0.00124
1
313.15
5
2
0.3228
4
3
0.1035
4
1
1.37242
6
1
0.00124
1
313.15
5
2
0.488
4
3
0.0174
3
1
1.36578
6
1
0.00124
1
313.15
5
2
0.488
4
3
0.0516
3
1
1.37285
6
1
0.00124
1
313.15
5
2
0.488
4
3
0.1035
4
1
1.37764
6
1
0.00124
1
318.15
5
2
0.3228
4
3
0.0174
3
1
1.35718
6
1
0.00124
1
318.15
5
2
0.3228
4
3
0.0516
3
1
1.36031
6
1
0.00124
1
318.15
5
2
0.3228
4
3
0.1035
4
1
1.36734
6
1
0.00125
1
318.15
5
2
0.488
4
3
0.0174
3
1
1.36227
6
1
0.00124
1
318.15
5
2
0.488
4
3
0.0516
3
1
1.36942
6
1
0.00124
1
318.15
5
2
0.488
4
3
0.1035
4
1
1.37418
6
1
0.00124
1
323.15
5
2
0.3228
4
3
0.0174
3
1
1.35309
6
1
0.00124
1
323.15
5
2
0.3228
4
3
0.0516
3
1
1.35702
6
1
0.00124
1
323.15
5
2
0.3228
4
3
0.1035
4
1
1.36166
6
1
0.00124
1
323.15
5
2
0.488
4
3
0.0174
3
1
1.35984
6
1
0.00124
1
323.15
5
2
0.488
4
3
0.0516
3
1
1.36664
6
1
0.00124
1
323.15
5
2
0.488
4
3
0.1035
4
1
1.37124
6
1
0.00124
1
333.15
5
2
0.3228
4
3
0.0174
3
1
1.34624
6
1
0.00124
1
333.15
5
2
0.3228
4
3
0.0516
3
1
1.35166
6
1
0.00124
1
333.15
5
2
0.3228
4
3
0.1035
4
1
1.35506
6
1
0.00124
1
333.15
5
2
0.488
4
3
0.0174
3
1
1.35502
6
1
0.00124
1
333.15
5
2
0.488
4
3
0.0516
3
1
1.36139
6
1
0.00124
1
333.15
5
2
0.488
4
3
0.1035
4
1
1.36743
6
1
0.00124
10
1
1
2
1
3
1
Principal objective of the work
JAB
TRC
8/19/2009
1
Mass density, kg/m3
VIBTUB:UFactor:16
Liquid
Direct value, X
1
Data file compiler
Propagation of evaluated standard uncertainties
95
Liquid
1
Pressure, kPa
Liquid
101
3
1
Temperature, K
Liquid
2
Mass fraction
1
Liquid
3
Mass fraction
2
Liquid
1
298.15
5
2
0.3228
4
3
0.0174
3
1
1024.783
7
1
0.662
1
298.15
5
2
0.3228
4
3
0.0516
3
1
1025.327
7
1
0.665
1
298.15
5
2
0.3228
4
3
0.1035
4
1
1026.382
7
1
0.672
1
298.15
5
2
0.488
4
3
0.0174
3
1
1036.829
7
1
0.745
1
298.15
5
2
0.488
4
3
0.0516
3
1
1037.365
7
1
0.748
1
298.15
5
2
0.488
4
3
0.1035
4
1
1038.328
7
1
0.754
1
303.15
5
2
0.3228
4
3
0.0174
3
1
1022.845
7
1
0.65
1
303.15
5
2
0.3228
4
3
0.0516
3
1
1023.638
7
1
0.655
1
303.15
5
2
0.3228
4
3
0.1035
4
1
1024.216
7
1
0.658
1
303.15
5
2
0.488
4
3
0.0174
3
1
1034.515
7
1
0.73
1
303.15
5
2
0.488
4
3
0.0516
3
1
1035.038
7
1
0.733
1
303.15
5
2
0.488
4
3
0.1035
4
1
1035.96
7
1
0.739
1
308.15
5
2
0.3228
4
3
0.0174
3
1
1020.478
7
1
0.635
1
308.15
5
2
0.3228
4
3
0.0516
3
1
1021.327
7
1
0.64
1
308.15
5
2
0.3228
4
3
0.1035
4
1
1022.135
7
1
0.645
1
308.15
5
2
0.488
4
3
0.0174
3
1
1032.086
7
1
0.715
1
308.15
5
2
0.488
4
3
0.0516
3
1
1032.595
7
1
0.718
1
308.15
5
2
0.488
4
3
0.1035
4
1
1033.48
7
1
0.724
1
313.15
5
2
0.3228
4
3
0.0174
3
1
1018.342
7
1
0.621
1
313.15
5
2
0.3228
4
3
0.0516
3
1
1018.923
7
1
0.625
1
313.15
5
2
0.3228
4
3
0.1035
4
1
1019.582
7
1
0.629
1
313.15
5
2
0.488
4
3
0.0174
3
1
1029.57
7
1
0.699
1
313.15
5
2
0.488
4
3
0.0516
3
1
1030.069
7
1
0.702
1
313.15
5
2
0.488
4
3
0.1035
4
1
1030.918
7
1
0.708
1
318.15
5
2
0.3228
4
3
0.0174
3
1
1015.946
7
1
0.606
1
318.15
5
2
0.3228
4
3
0.0516
3
1
1016.452
7
1
0.61
1
318.15
5
2
0.3228
4
3
0.1035
4
1
1017.222
7
1
0.614
1
318.15
5
2
0.488
4
3
0.0174
3
1
1026.868
7
1
0.682
1
318.15
5
2
0.488
4
3
0.0516
3
1
1027.357
7
1
0.685
1
318.15
5
2
0.488
4
3
0.1035
4
1
1028.172
7
1
0.69
1
323.15
5
2
0.3228
4
3
0.0174
3
1
1013.41
7
1
0.591
1
323.15
5
2
0.3228
4
3
0.0516
3
1
1013.896
7
1
0.594
1
323.15
5
2
0.3228
4
3
0.1035
4
1
1014.68
7
1
0.599
1
323.15
5
2
0.488
4
3
0.0174
3
1
1024.008
7
1
0.664
1
323.15
5
2
0.488
4
3
0.0516
3
1
1024.487
7
1
0.667
1
323.15
5
2
0.488
4
3
0.1035
4
1
1025.274
7
1
0.672
1
328.15
5
2
0.3228
4
3
0.0174
3
1
1010.647
7
1
0.573
1
328.15
5
2
0.3228
4
3
0.0516
3
1
1011.128
7
1
0.576
1
328.15
5
2
0.3228
4
3
0.1035
4
1
1011.882
7
1
0.581
1
328.15
5
2
0.488
4
3
0.0174
3
1
1021.093
7
1
0.646
1
328.15
5
2
0.488
4
3
0.0516
3
1
1021.576
7
1
0.649
1
328.15
5
2
0.488
4
3
0.1035
4
1
1022.335
7
1
0.654
1
333.15
5
2
0.3228
4
3
0.0174
3
1
1007.861
7
1
0.556
1
333.15
5
2
0.3228
4
3
0.0516
3
1
1008.326
7
1
0.559
1
333.15
5
2
0.3228
4
3
0.1035
4
1
1008.763
7
1
0.562
1
333.15
5
2
0.488
4
3
0.0174
3
1
1018.037
7
1
0.627
1
333.15
5
2
0.488
4
3
0.0516
3
1
1018.498
7
1
0.63
1
333.15
5
2
0.488
4
3
0.1035
4
1
1018.942
7
1
0.633
1
338.15
5
2
0.3228
4
3
0.0174
3
1
1004.814
7
1
0.537
1
338.15
5
2
0.3228
4
3
0.0516
3
1
1005.21
7
1
0.54
1
338.15
5
2
0.3228
4
3
0.1035
4
1
1005.946
7
1
0.544
1
338.15
5
2
0.488
4
3
0.0174
3
1
1014.921
7
1
0.608
1
338.15
5
2
0.488
4
3
0.0516
3
1
1015.341
7
1
0.61
1
338.15
5
2
0.488
4
3
0.1035
4
1
1016.063
7
1
0.615